Carbon dioxide geological storage potential in saline aquifer of sedimentary basins in China Sea
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摘要:
二氧化碳地质封存是二氧化碳捕集利用封存（CCUS）技术的关键环节，海域二氧化碳地质封存是将工业碳排放源或油气开发过程中捕集的二氧化碳，以超临界态注入到海底咸水层、废弃或开发中油气藏等地质体中，实现与大气长期隔离的过程。因远离人类居住地且有海水覆盖、具有“安全性高、环境风险小”特点，海域二氧化碳地质封存受到欧美等国家和地区的高度重视。本文在分析我国海域沉积盆地基本地质条件基础上，采用创新的模型体积法评价了我国海域沉积盆地咸水层二氧化碳地质封存潜力。研究表明，我国海域沉积盆地新生界厚度大，地壳稳定性较好，具有中低地温场特征，发育多套储碳-封盖组合，构造地层圈闭多，二氧化碳地质封存条件优越、咸水层封存潜力巨大。这将为我国海洋地质碳封存区带评价和目标区优选提供依据，对我国沿海省市碳达峰碳中和路径规划和离岸碳封存示范工程预研究具有重要意义。
Abstract:Geological storage of carbon dioxide is the key link of carbon dioxide capture, utilization and storage (CCUS) technology. Marine carbon dioxide geological storage is the process of injecting supercritical carbon dioxide captured by industrial carbon emission sources or oil and gas development into geological bodies, such as seabed salt water layers, abandoned or developing oil and gas reservoirs, to achieve long-term isolation from the atmosphere. Because it is far from human habitation and covered by sea water, it has the characteristics of "high safety and low environmental risk", the geological storage of Marine carbon dioxide has been highly valued by European and American countries and regions. Based on the analysis of the basic geological conditions of sedimentary basins in China Sea area, an innovative model volume method is used to evaluate the geological storage potential of carbon dioxide in brackish layers of sedimentary basins in China Sea area. The analysis shows that the sedimentary basins in the sea area of China have large Cenozoic thickness, good crustal stability, characteristics of middle and low geothermal field, multiple sets of carbon storage and capping combinations, more structural and stratigraphic traps, superior geological conditions for carbon dioxide storage, and great potential for salt water reservoir storage. This will provide a basis for the evaluation of marine carbon dioxide geological storage zones and the optimization of target areas, and has great significance for the path planning of carbon peaking carbon neutrality and the pre-study of offshore carbon dioxide geological storage demonstration projects in China's coastal provinces and cities.
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表 1 中国海域主要沉积盆地地质特征
Table 1. Geological characteristics of major sedimentary basins in China Sea
盆地名称 评价面积/km2 新生界厚度/m 水深/m 地温梯度/(℃/km) 大地热流值/(mW/m2) 范围/平均值 范围/平均值 范围/平均值 渤海盆地 54 476 200～7 000 0～55/18 28～43/30 50～85/65.5 北黄海盆地 16 401 200～3 800 23～80/51 23～28/25 无数据 南黄海盆地 136 361 600～6 000 1～114/53 24～30/29.3 61～66/63.5 东海陆架盆地 239 580 2 250～17 500 4～894/97 24～50/30 50～88/68 冲绳海槽盆地 147 963 800～8 000 0～2493/919 8～194/80.68 9～437/96.2 台湾海峡盆地 22 565 400～5 000 0～92/52 39～45/41 无数据 台西南盆地 42 185 400～10 700 0～3 385/1 288 33～47/39 3～170/65.6 珠江口盆地 200 136 400～9 000 0～2919/439 29～113/42 59～81/69.95 北部湾盆地 52 222 400～5 000 0～91/31 35～39/37.5 62～68/64.67 琼东南盆地 96 289 500～14 000 4～2 970/1 054 25.2～60.8/40 83～112/95.7 莺歌海盆地 114 785 2 070～18 000 0～645/73 31～43/40 69～117/85 中建南盆地 134 497 1 400～8 000 16～4 343/1 815 /35 无数据 曾母盆地 217 268 2 000～18 000 0～1 796/224 25～50/46 60～120/90.9 北康盆地 78 499 1 000～12 000 0～2 746/1 539 30～40/34 43.9～45.1/44.5 南安盆地 191 703 2 000～12 000 0～3 387/959 21～38/29 46～80/55.7 文莱沙巴盆地 65 632 3 500～12 000 0～2 200/400 18.2～32.5/28 51～72/60.5 礼乐盆地 74 950 1 800～5 700 0～3 553/1 333 /29 23～26/24.5 巴拉望盆地 48 044 3 000～8 000 0～3 826/833 22～41/33 35～83/54.2 
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表 2 海域沉积盆地咸水层二氧化碳地质封存潜力
Table 2. Geologic storage potential of carbon dioxide in saline aquifers of maritime sedimentary basins
序号 盆地 预测潜力/108 t E1=1.2% E2=2.4% E3=4.1% 1 渤海盆地 754 1 508 2 576 2 珠江口盆地 1 248 2 496 4 265 3 东海陆架盆地 1 629 3 259 5 567 4 北部湾盆地 228 456 779 5 莺歌海盆地 303 606 1 036 6 琼东南盆地 1 307 2 615 4 467 7 南黄海盆地 932 1 863 3 183 8 台西南盆地 424 847 1 448 9 台湾海峡盆地 90 181 309 10 北黄海盆地 43 86 147 11 中建南盆地 661 1 323 2 260 12 北康盆地 1 037 2 075 3 545 13 南安盆地 1 903 3 806 6 502 14 曾母盆地 1 050 2 101 3 589 15 冲绳海槽盆地 524 1 048 1 790 16 礼乐盆地 268 536 915 17 文莱沙巴盆地 342 685 1 170 18 巴拉望盆地 160 321 548 总计 12 903 25 812 44 096 注：E1、E2、E3分别为置信度90%、50%、10%的二氧化碳封存有效系数
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